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Please use this identifier to cite or link to this item: http://hdl.handle.net/2241/98262

Title: Exciton localization and decomposition dynamics in cuprous halide nanocrystals
Authors: Okuno, Tsuyoshi
Miyajima, Hiroshi
Satake, Akihiro
Masumoto, Yasuaki
舛本, 泰章
Issue Date: Dec-1996
Publisher: American Physical Society
Journal Title: Physical review B
Volume: 54
Issue: 23
Start Page: 16952
End Page: 16957
DOI: 10.1103/PhysRevB.54.16952
PMID: 9985824
Abstract: We report temporal changes of luminescence and absorption (differential transmission) of excitons in nanometer-size semiconductor crystals (nanocrystals) of CuCl embedded in NaCl or in glass, and CuBr nano- crystals embedded in glass. In CuCl nanocrystals in NaCl, an exciton relaxes nonradiatively to some localized state. In CuCl and CuBr nanocrystals in glass, the temporal changes of the differential transmission have a longer decay component in addition to the fast decay component which agrees with the luminescence decay. This result suggests exciton decomposition and the existence of an electron or a hole remainder in the nano- crystals. The decay time of the longer decay component increases by the accumulation of photoexcitation. This phenomenon indicates persistent trapping of carriers in the glass matrix, which is concerned with persistent spectral hole burning in nanocrystals.
URI: http://hdl.handle.net/2241/98262
Rights: ©1996 The American Physical Society
Text Version: publisher
Appears in Collections:Physical review B
舛本 泰章 (Masumoto Yasuaki)

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